New PDF release: Electroanalytical Chemistry: A Series of Advances, Vol. 22

By Allen J. Bard, Israel Rubinstein

ISBN-10: 0824747194

ISBN-13: 9780824747190

ISBN-10: 0824757858

ISBN-13: 9780824757854

For greater than 3 many years the Electroanalytical Chemistry sequence has brought the main in-depth and significant examine with regards to matters in electrochemistry.  Volume 22 keeps this gold-standard with sensible stories of modern purposes, in addition to cutting edge contributions from the world over revered specialists—highlighting the emergence of recent applied sciences and traits within the box. prior volumes within the sequence have been “highly advised” via the magazine of the yankee Chemical Society and regarded “essential” through the magazine of sturdy kingdom Electrochemistry, and this quantity maintains with a set of state of the art advances and experiences of the top quality.

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Extra resources for Electroanalytical Chemistry: A Series of Advances, Vol. 22

Sample text

The derivation of such a model is complicated by the fact that electro-neutrality does not exist on the solution side of the interface (except at the potential of zero charge), although the electrostatic energy is reduced by interaction with the image charges on the metal side of the interface. D. 1. Quartz Crystals with Rough Surfaces Quartz Crystals with Rough Surfaces Operating in Liquids When the surface of quartz crystal resonator is rough, the liquid motion generated by the oscillating surface becomes much more complicated than for the smooth surface.

40 Tsionsky et al. The remaining part of the overall effect can then be ascribed to viscosity effect, gf. Using pairs of experimental data Df vs. E, and the dependence of surface charge density on potential, the concentration of ions (Ca,c) in the diffuse double layer can be calculated and the dependence of gf on Ca,c can be obtained. An example of such calculations is shown in Fig. 7 [61,97]. Some specific features of the data shown here merit special attention: 1. At negative rational potentials, where the diffuse double layer is populated mostly by K+ ions, the dependence of gf on concentration for solutions of KOH and KNO3 coincided.

Using such values, the added weight of anions adsorbed electrostatically in the diffuse double layer can be evaluated. The solid lines in Fig. 6 show the results of these calculations. It is clearly seen that these lines do not fit the experiments. Moreover, electrostatic adsorption alone predicts the maximum EQCM frequency always at the pzc, while the experimentally observed position of the maximum depends on the composition of the solution. c. Viscosity Effect in the Diffuse Double Layer A difference between the viscosity of the fluid in the diffuse double layer and in the bulk of the solution could be caused by two factors.

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Electroanalytical Chemistry: A Series of Advances, Vol. 22 by Allen J. Bard, Israel Rubinstein

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