Get Characterization of Porous Solids II PDF

By F. Rodriguez-Reinoso, J. Rouquerol, K. S. W. Sing

ISBN-10: 0080887481

ISBN-13: 9780080887487

ISBN-10: 0444885692

ISBN-13: 9780444885692

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The calculation of the supercritical adsorption of LJ methane in carbon pores suggests that there exists an optimum pore size for methane adsorbed in porous carbon. At a fixed temperature, the maximum excess adsorption per unit of pore volume passes through a global maximum for a particular pore width. The selectivity isotherm for methane-ethane mixtures shows different shapes when the temperature changes. At high temperatures, it passes through a maximum. When the temperature is near the capillary critical one, a second maximum appears.

2 . E. Gubbins, F. van Swol and U. Marini Bettolo Marconi, Mixtures confined to narrow slit pores: Computer simulation and theory, Proc. Third Internat. Conf. on Fund. , Sonthofen, FRG, in press (1990). 2 . Tan, F. E. Gubbins, Lennard-Jones mixtures in cylindrical pores, Molec. , 62, 1213 (1987). A. Steele, The physical interactionof gases with crystalline solids, Surf. , 36, 317 (1973); The interaction of gases with solid surfaces, Pergamon, Oxford (1974). F. Rodriguez-Reinoso et al. , Amsterdam 31 SORPTION OF GASES ON MICROPOROUS SOLIDS: PORE SIZE CHARACTERIZATION BY GAS SORPTION STEVEN W.

2. In the SDA results in Figs. 0 P/P" Fig. 35. - Fig. 95. The metastable regions predicted by the SDA are included. 25 dependent hard sphere diameter was used [12]. Good agreement between the SDA and computer simulation is found in both cases. In Fig. 3 , we compare the LDA, SDA, and Kelvin equation with molecular dynamics (MD) simulation results for LJ fluids in cylindrical pores using the results of Peterson et al. [3]. The Kelvin equation is where po is bulk fluid vapor pressure, y and vL are the surface tension and molar volume of the liquid, N is Avogadro's number, k is Boltzmann's constant, and R is pore radius.

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Characterization of Porous Solids II by F. Rodriguez-Reinoso, J. Rouquerol, K. S. W. Sing

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