Download e-book for kindle: C-H Activation by Andrew Martins, Brian Mariampillai, Mark Lautens (auth.),

By Andrew Martins, Brian Mariampillai, Mark Lautens (auth.), Jin-Quan Yu, Zhangjie Shi (eds.)

ISBN-10: 3642123554

ISBN-13: 9783642123559

Table of Contents - Synthesis within the Key of Catellani: Norbornene-Mediated ortho C–H Functionalization - Mechanistic issues within the improvement and Use of Azine, Diazine and Azole N-Oxides in Palladium-Catalyzed Direct Arylation - Palladium and Copper Catalysis in Regioselective, Intermolecular Coupling of C–H and C–Hal Bonds - Pd-Catalyzed C–H Bond Functionalization at the Indole and Pyrrole Nucleus - distant C–H Activation through Through-Space Palladium and Rhodium Migrations - Palladium-Catalyzed Aryl–Aryl Bond Formation via Double C–H Activation - Palladium-Catalyzed Allylic C–H Bond Functionalization of Olefins - Ruthenium-Catalyzed Direct Arylations via C–H Bond Cleavages - Rhodium-Catalyzed C–H Bond Arylationof Arenes - Cross-Dehydrogenative Coupling Reactions of sp3-Hybridized C–H Bonds - Functionalization of Carbon–Hydrogen Bonds via Transition steel Carbenoid Insertion - Metal-Catalyzed Oxidations of C–H to C–N Bonds

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1 Synthetic Considerations . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2 Reactivity with Azine and Diazine N-Oxides . . . . . . . . . . . . . . . . . . . . . 3 Regioselectivity with Nonsymmetrical Azine Substrates . . . . . . . . . . . . . . . 4 Azole N-Oxides . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5 Methods for N-Oxide Deoxygenation .

53 References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 54 K. ca 36 K. 1 Biaryl Compounds in Nature and Medicinal Chemistry The biaryl structural motif is prevalent in natural products and in pharmaceutical and material sciences ([1–4]; for a review on P, N ligands with pyridyl donors see [5, 6]). While chemists often find inspiration in the methods nature employs to create molecular architectures, the techniques used by nature to form biaryls offer little guidance for the majority of aromatic targets whose synthesis is required of organic chemists.

53 References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 54 K. ca 36 K. 1 Biaryl Compounds in Nature and Medicinal Chemistry The biaryl structural motif is prevalent in natural products and in pharmaceutical and material sciences ([1–4]; for a review on P, N ligands with pyridyl donors see [5, 6]). While chemists often find inspiration in the methods nature employs to create molecular architectures, the techniques used by nature to form biaryls offer little guidance for the majority of aromatic targets whose synthesis is required of organic chemists.

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C-H Activation by Andrew Martins, Brian Mariampillai, Mark Lautens (auth.), Jin-Quan Yu, Zhangjie Shi (eds.)


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